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The 1st NATO technology discussion board used to be held in Biarritz in September 1990. This Taormina convention is the second one in a chain that we want to be an extended one and that i think that it has equalled the good fortune of its predecessor. In establishing those conferences the NATO technological know-how Committee desired to assemble major specialists to study fields of sturdy current curiosity.
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As we study the template that created the Borromean link or as we puzzle over the fate and/or uses of Vögtle’s dendrimerized knotanes- (perhaps serving as chiral tectons) we are like mountain climbers following a well-marked trail up to misty heights, but without the struggles of the first pioneering effort to reach those heights. History has value to researchers for many reasons: detailed knowledge accumulates and what was learned, if it was true, it still is true; it can inspire us and provide a basis for celebrating the advances of our fields; it can humanize our necessarily uncompromising encounter with experimental reality; it can guide us to not make the kinds of mistakes made by others; it shows us that the seemingly impossible challenges of today become the records of accomplishment in time.
A) Ogina H (1981) J Am Chem Soc 103:1303; b) Yamanari K, Shimura Y (1983) Bull Chem Soc Jpn 56:2283 32. Kim K (2002) Chem Soc Rev 31:96 33. Mock WL, Shih N-Y (1986) J Org Chem 51:4440 34. Busch DH, Burke JA, Jicha DC, Thompson MC, Morris ML (1963) Adv Chem Series 37:125 35. Schrauzer GN (1962) Ber 95:1438; Umland F, Thierig D (1962) Angew Chem 74:388 36. Curry JD, Busch DH (1964) J Am Chem Soc 86:592 37. a) Melson GA, Busch DH (1963) Proc Chem Soc 1963:223; b) Melson GA, Busch DH (1964) J Am Chem Soc 86:4830; c) Melson GA, Busch DH (1964) J Am Chem Soc 86:4834; d) Melson GA, Busch DH (1964) J Am Chem Soc 87:1706 38.
If rotaxanes were, at first, difficult to make, higher rotaxanes were a great challenge and this too has been overcome. Hydrogen-bonded templates provide good examples of the relative difficulty of synthesizing both - and rotaxanes. Stoddart and his collaborators used 1,2,3-triazole stoppered secondary ammonium axles and a symmetrical 1,4-phenylene linked 28crown8  to produce - and rotaxanes in yields of 30% and 10%, respectively, a difference that reflects the relative difficulty of rotaxane synthesis.