By Henderson W. E.
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The addition of five d orbitals to an s and p set, either as extra orbitals in the second period (the third row) from silicium to chlorine, or as valence orbitals for transition metal complexes is taking into account straightforwardly by raising the dimensions of the block matrices up to nine . However, mixing the d functions added to the valence orbitals of nonmetals, for instance sulphur, or keeping them in their primitive form, has not a great importance, because they play just a role of polarization functions in molecular structure calculations using hybridization .